Reactions of Halogen Oxides Studied by Flash Photolysis. IV. Vacuum Ultraviolet Kinetic Spectroscopy Studies on Chlorine Dioxide

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Scientific paper

The rate constants for the production of vibrationally excited oxygen in the reactions O + ClO2 -> O2(\upsilon ' '<= 15) + ClO O + ClO -> O2(\upsilon ' '<= 14) + Cl are approximately equal for all values of \upsilon ' '<= 13. The oxygen initially receives 45 ± 10% of the heat of reaction in the form of vibrational energy. Extinction coefficients have been measured for several bands of the C-X, D-X and E-X systems of ClO2 in the vacuum ultraviolet. Five new systems are reported between 141 and 128 nm. Two of these, F-X and J-X, and the C-X system form a Rydberg series for an ionization potential of 10.36 eV.

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