On the photofragmentation of SF$_2^+$: Experimental evidence for a predissociation channel

Details On the photofragmentation of SF$_2^+$: Experimental evidence for a predissociation channel On the photofragmentation of SF$_2^+$: Experimental evidence for a predissociation channel

2008-08-19

arxiv.org/abs/0808.2622v3

JCP 129, 166101 (2008).

Physics

Chemical Physics

7 pages, 3 figures, submitted to JCP as a Note

Scientific paper

10.1063/1.3000006

We report on the first observation of the photofragmentation dynamics of SF$_2^+$. With the aid of state-of-the-art ab initio calculations on the low-lying excited cationic states of SF$_2^+$ performed by Lee et al. [J. Chem. Phys. 125, 104304 (2006)], a predissociation channel of SF$_2^+$ is evidenced by means of resonance-enhanced multilphoton ionization spectroscopy. This work represents a second experimental investigation on the low-lying excited cationic states of SF$_2^+$. [The first one is the He I photoelectron spectrum of SF$_2^+$ reported by de Leeuw et al. three decades ago, see Chem. Phys. 34, 287 (1978).]

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