Uncertainties in reactive uptake coefficients for solid stratospheric particles-1. Surface chemistry

Details Uncertainties in reactive uptake coefficients for solid stratospheric particles-1. Surface chemistry Uncertainties in reactive uptake coefficients for solid stratospheric particles-1. Surface chemistry

Jul 1997

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1997georl..24.1743c&link_type=abstract

Geophysical Research Letters, Volume 24, Issue 14, p. 1743-1746

Physics

22

Atmospheric Composition And Structure, Atmospheric Composition And Structure: Aerosols And Particles, Atmospheric Composition And Structure: Chemical Kinetic And Photochemical Properties, Atmospheric Composition And Structure: Cloud Physics And Chemistry

Scientific paper

Laboratory data for reactions of ClONO2 or HOCl with HCl on nitric acid trihydrate and sulfuric acid tetrahydrate are compared using a surface reaction model. Data sets where both non-reactive and reactive uptake were measured reveal that changes in the reactive uptake coefficients of ClONO2 and HOCl can be explained completely by the amount of HCl taken up by the hydrates. Large discrepancies are revealed between measurements from different laboratories which have important consequences for calculated ozone destruction (see companion paper II).

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