Actinide microdistributions in the enstatite meteorites

Mathematics – Logic

Scientific paper

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Actinide Series, Chondrites, Enstatite, Meteoritic Composition, Radioactive Age Determination, Calcium Sulfides, Fractionation, Mineralogy, Plutonium 244, Thorium, Uranium 238

Scientific paper

The results of measurements of the mineralogical distribution of Th, U, and Pu-244 in the enstatite meteorites are reported. The obtained information is used to define the behavior of Th and U under highly reducing conditions, evaluate the reported variation of Th/U in enstatite chondrites, and evaluate the suitability of enstatite meteorites for Pu-244/U-238 chronology. For the E-6 chrondrites it is found that the main reservoir for Th and U is oldhamite, which has mean Th and U abundances of 1550 + or - 80 ppb Th and 410 + or - 20 ppb U. For E-5 chondrite, only oldhamite is found to contain substantial quantities of Th and U, while E-4 niningerite contains 45 + or - 5 ppb U. Oldhamite from E-5 and E-4 shows actinide enrichments but at levels about half the E-6 results. A lack of Th-U fractionation is evident in both the oldhamite and the meteorites themselves, which suggests that the enstatite chondrites may be well-suited for Pu-U chronology and for providing the initial Pu-U value in the early solar system.

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