Microwave spectra of van der Waals complexes of importance in planetary atmospheres

Computer Science

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Bonding, Microwave Spectra, Planetary Atmospheres, Rotational Spectra, Splitting, Van Der Waals Forces, Dimers, Fabry-Perot Spectrometers, Microwave Spectrometers, Trimers

Scientific paper

The Fourier-transform Fabry-Perot pulsed-molecular-beam microwave spectrometer at NIST was used to study the microwave spectra of a number of molecular dimers and trimers that may be present in planetary atmospheres. The weak van der Waals bonds associated with these species usually give rise to rotational-tunneling splittings in the microwave spectra. The microwave spectrum of the water dimer species was used to illustrate the complications that can arise in the study of the rotational spectra of these loosely bound species. In addition to the water dimer species, the microwave spectra of the following hydrogen-bonded and van der Waals complexes were studied: (CO2)2-H2O, CO2-(H2O)2, CO2-H2S, N2-H2O, CO-H2O, SO2-H2O, and O3-H2O.

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