Other
Scientific paper
Mar 1974
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1974gecoa..38..453f&link_type=abstract
Geochimica et Cosmochimica Acta, vol. 38, Issue 3, pp.453-470
Other
6
Scientific paper
Dehydration of Orgueil by stepwise calcination produced more than a tenfold change in its Kr B.E.T. surface area, which increased to 120 m 2 /g, then fell to 40 m 2 /g. This phenomenon characterizes structures of the montmorillonite type, but not other plausible constituents of Orgueil. It results from vacating of interlayer sites by H 2 O molecules which are replaced by Kr until finally the sheets collapse, excluding Kr. Differential calorimetric scans of Orgueil also gave a better match for montmorillonite than for other minerals. However, a simple identification as montmorillonite conflicts with chemical analyses of Orgueil phyllosilicates. Exchangeability of H 2 O in Orgueil was shown by water regain from lab air between calcination cycles and similarily of the cycles. Room temperature dehydration revealed up to 6 per cent free surface adsorbed water. High D/H ratios in CI's may result from D enrichment in OH - groups during equilibration of dispersed phyllosilicate dust with nebula gas at temperatures <<0°C. Adsorption on the very large free and interlayer surface areas of this dust was the major mechanism by which volatiles still uncondensed at the time of gas-dust separation (including planetary primordial Ar, Kr and Xe) were incorporated into solid solar system material.
Cannon W. A.
Fanale Fraser P.
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