Can phase space theory reproduce experimental neutral product branching ratios for dissociative recombination reactions?

Details Can phase space theory reproduce experimental neutral product branching ratios for dissociative recombination reactions? Can phase space theory reproduce experimental neutral product branching ratios for dissociative recombination reactions?

Aug 1991

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1991apj...376..531g&link_type=abstract

Astrophysical Journal, Part 1 (ISSN 0004-637X), vol. 376, Aug. 1, 1991, p. 531-539. Research supported by NSF.

Astronomy and Astrophysics

Astrophysics

23

Cosmochemistry, Interstellar Matter, Molecular Clouds, Chemical Evolution, Hydrogen Atoms, Recombination Reactions

Scientific paper

A formulation of the statistical phase space theory has been used to obtain neutral product branching ratios for tetratomic ion-electron dissociative recombination reactions. The results have been compared with recent experimental results for the H3O(+) + e, NNOH(+) + e, HOCO(+) + e, AND H3S(+) + e reactions. Two conclusions have been reached. First, some dissociative recombination reactions can be described by a phase space theory that contains neutral product distributions with limited rotational excitation. Second, phase space theory does not currently possess general predictive power, free from parameterization, for tetratomic ion-electron dissociative recombination reactions.

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