High Resolution Sub-Millimeter Spectroscopic Studies of Iron-Containing Free Radicals

Details High Resolution Sub-Millimeter Spectroscopic Studies of Iron-Containing Free Radicals High Resolution Sub-Millimeter Spectroscopic Studies of Iron-Containing Free Radicals

Sep 1997

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1997phdt.........6a&link_type=abstract

Thesis (PHD). ARIZONA STATE UNIVERSITY , Source DAI-B 58/03, p. 1302, Sep 1997, 241 pages.

Computer Science

Scientific paper

High resolution millimeter/sub-millimeter-wave spectroscopic studies were performed on several gas phase iron containing free radicals using a newly designed and constructed spectrometer. Spectroscopic parameters such as rotational, fine structure, magnetic hyperfine structure, electric quadrupole, and lambda-type doubling constants were determined, using a non-linear least-squares fitting routine of an effective Hamiltonian. The interpretation of these parameters has resulted in an increased understanding of structural and bonding characteristics of iron-containing species. The experimentally determined parameters and bond lengths have been compared with previous experimental results and ab initio calculations when available.

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