Temperature dependence of infrared bands produced by polycyclic aromatic hydrocarbons

Astronomy and Astrophysics – Astrophysics

Scientific paper

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Aromatic Compounds, Cyclic Hydrocarbons, Infrared Spectra, Interstellar Matter, Infrared Absorption, Temperature Dependence

Scientific paper

The behavior of IR absorption bands with temperature has been examined systematically in the laboratory for three representative polycyclic aromatic hydrocarbon molecules: coronene, chrysene, and 1-methylcoronene. A careful description of both intensity and profile measured for most of the bands is reported. A tentative interpretation of the observed variations is given in terms of extra-molecular effects produced by the anharmonicity of the vibrational energy levels as a function of temperature. These new laboratory data provide an accurate description of the optical properties for representative molecules often used to account for the so-called unidentified infrared bands emitted by astronomical sources.

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