Water and magmas: application of the Gibbs-Duhem equation

Details Water and magmas: application of the Gibbs-Duhem equation Water and magmas: application of the Gibbs-Duhem equation

Mar 1978

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1978gecoa..42..275d&link_type=abstract

Geochimica et Cosmochimica Acta, vol. 42, Issue 3, pp.275-276

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(1975a, b) has shown that in several alumino-silicate systems Henry's law constant is independent of silicate melt composition up to X melt H 2 O = 0.5. He has used this fact to conclude that such silicate melts behave ideally over a wide range of compositions based on the application of the Gibbs-Duhem relation. Unless Henry's law is valid up to X melt H 2 O = 1.0, the application of the Gibbs--Duhem relation to three component systems only shows that if one component obeys Henry's law, the other two components follow the two component Gibbs-Duhem equation. There is no thermodynamic requirement of ideality.

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