Mathematics – Logic
Scientific paper
Jun 2010
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2010mss..confetc09w&link_type=abstract
"International Symposium On Molecular Spectroscopy, 65th Meeting, Held 21-25 June, 2010 at Ohio State University. http://molspec
Mathematics
Logic
Microwave (Rotational)
Scientific paper
Two-dimensional broadband techniques have been introduced into the microwave regime using chirped-pulse Fourier transform spectroscopy. Theoretical considerations of expanding the prototypical three-level model to an N-level system are presented. Representative Hamiltonian and density matrices were used to solve the Liouville-von Neumann equations of motion in order to describe the evolution of coherently prepared states. Several selective excitation pulse sequences were performed on 1-chloro-1-fluoroethylene and 3,3,3-trifluoropropyne to test the validity of the theory. Through modeling one-dimensional slices of a traditional 2D plot, peaks in the indirectly measured frequency dimension were identified and classified and phenomenological selection rules were obtained.
Dian Brian C.
Hotopp Kelly M.
Shirar Amanda J.
Wilcox David S.
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