Time-resolved Electron Impact Study of Excitation of H2 Singlet-Gerade States from Cascade Emission in the Vacuum Ultraviolet Region

Astronomy and Astrophysics – Astronomy

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Methods: Laboratory, Molecular Data, Molecular Processes

Scientific paper

Medium-resolution (full width at half-maximum Δλ=0.5 Å) vacuum ultraviolet (VUV) emission spectra of H2 from forbidden excitation to the excited singlet-gerade states and subsequent cascade to the singlet-ungerade states have been studied with a time-resolved electron-impact technique. Emissions from the B 1Σ+u, C 1Πu, B' 1Σ+u, and D 1Πu states that are entirely due to cascade from the singlet-gerade states have been observed. Lyman band emission intensities dominate over the entire 940-1650 Å wavelength region, though Werner band emission intensities are also significant. In addition, very weak cascade emissions from the vj=0 and 1 levels of the B' 1Σ+u and D 1Πu states are also evident. In contrast to previous assumption, the cascade excitation is observed to take place over all the vibrational levels of the B 1Σ+u and C 1Πu states, while contributing heavily to low vj levels of the B 1Σ+u state. Synthetic spectra based on the calculated transition probabilities of the EF 1Σ+g, GK 1Σ+g, HH 1Σ+g, I 1Πg, J 1Δg, O 1Σ+g and P 1Σ+g-->B 1Σ+u, C 1Πu, B' 1Σ+u, and D 1Πu band systems and Franck-Condon factors of the EF 1Σ+g-X 1Σ+g, GK 1Σ+g-X 1Σ+g, HH 1Σ+g-X 1Σ+g, I 1Πg-X 1Σ+g, J 1Δg-X 1Σ+g, O 1Σ+g-X 1Σ+g, and P 1Σ+g-X 1Σ+g are in good agreement with the observed Lyman and Werner band intensities. The present study shows that a number of singlet-gerade and singlet-ungerade states are involved in the cascade excitation process of H2. The cascade from these states in the VUV provide diagnostic information on astrophysical sources for H2 emission.

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