Other
Scientific paper
Apr 1989
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1989gecoa..53..765m&link_type=abstract
Geochimica et Cosmochimica Acta, vol. 53, Issue 4, pp.765-771
Other
5
Scientific paper
The O-H stretching region (2800-3800 cm -1 ) in Raman spectra of aqueous solutions is sensitive to changes in the salt concentration. This permits determination of the salinity in the aqueous phase of fluid inclusions (at room temperature) by calculating skewing parameters from Raman microprobe spectra. The technique does not require detailed knowledge of the fluid composition and can be applied to most chloride solutions which commonly occur in fluid inclusions. Studies of synthetic fluid inclusions from the NaCl-H 2 O system show that salinities up to halite saturation may be determined to within ±2 wt%. Well-characterised fluid inclusions from the unconformity-related uranium deposits of Nabarlek and Koongarra, Northern Territory, Australia, were studied with the laser Raman microprobe. The salinities determined from the Raman spectra are comparable to those obtained using standard microthermometric techniques. The Raman microprobe technique has the advantage of not requiring analogy to binary salt-water phase diagrams which cannot adequately model the complex brines in these inclusions. Variations in the concentration of salt hydrates, observed in Raman spectra of frozen inclusions, validated the salinities derived from the Raman skewing parameters obtained at room temperature. The Raman analyses confirm previous microthermometric evidence for trapping of discrete high and low salinity fluids.
Mernagh T. P.
Wilde A. R.
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