Production of Doubly Charged Helium Ions by Two-Photon Absorption of an Intense Sub-10-fs Soft X-Ray Pulse at 42eV Photon Energy

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Photoionization Of Atoms And Ions, Strong-Field Excitation Of Optical Transitions In Quantum Systems, Multiphoton Processes, Dynamic Stark Shift, Ultrafast Processes, Optical Pulse Generation And Pulse Compression

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We report on the observation of doubly charged helium ions produced by a nonlinear interaction between a helium atom and photons with a photon energy of 42eV which are generated with the 27th harmonic of a femtosecond pulse from a Ti:sapphire laser. The number of ions is proportional to the square of the intensity of the 27th harmonic pulse, and thus two-photon double ionization should be dominantly induced as compared with other nonlinear processes accompanying sequential ionization via a singly charged ion. This phenomenon is utilized to measure the pulse duration of the 27th harmonic pulse by using an autocorrelation technique, for the first time to our knowledge, and as a result a duration of 8fs is found.

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