Phase control of a two-photon transition with shaped femtosecond laser-pulse sequences

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Coherent Control Of Atomic Interactions With Photons, Ultrafast Processes, Optical Pulse Generation And Pulse Compression, Other Multiphoton Processes

Scientific paper

Phase effects in a quantum control experiment on the two-photon transition 4s ←← 3s of atomic sodium are studied. In our experiment, we combine the generation of phase-locked interferometrically generated pulses with pulse-shaping techniques to study in detail the interplay of optical and quantum-mechanical phases. Subtle differences in the physical realization of the pulse sequences produce large difference in the control objective—the 4s population. The control mechanisms of more complex pulse sequences generated by periodic and discontinuous phase-modulation functions are investigated systematically and analyzed on the basis of quantum-mechanical interference.

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