Microwave Spectra and Structure of N_2 CO_2

Details Microwave Spectra and Structure of N_2 CO_2 Microwave Spectra and Structure of N_2 CO_2

Jun 2010

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2010mss..confeth01f&link_type=abstract

"International Symposium On Molecular Spectroscopy, 65th Meeting, Held 21-25 June, 2010 at Ohio State University. http://molspec

Computer Science

Microwave (Rotational)

Scientific paper

We present here the FTMW spectra of the various isotopologues of the weakly-bound complex of carbon dioxide with the most abundant molecule in the atmosphere, nitrogen. The structure of the complex along with the inversion of the N_2 (or lack of it) will be discussed. The molecule is T-shaped, with the OCO forming the cross of the T, a structure deduced from a previous rotationally-resolved infrared experiment. A significant wide-amplitude bending motion of the N_2 is deduced from the values of the (nearly identical) nuclear quadrupole coupling constants of the nitrogen nuclei. The spectroscopic results will be compared with ab-initio calculations. We will examine the consequences of N_2-CO_2 formation upon atmospheric opacity.
M. A. Walsh, T. R. Dyke, B. J. Howard, J. Mol. Struct. 189, 111-120 (1988)

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