Measurement of the stratospheric hydrogen peroxide concentration profile using far infrared thermal emission spectroscopy

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Atmospheric Composition, Balloon Sounding, Hydrogen Peroxide, Infrared Spectroscopy, Stratosphere, Thermal Emission, Data Processing, Data Reduction, Far Infrared Radiation, Fourier Transformation

Scientific paper

The first unequivocal measurement of hydrogen peroxide in the stratosphere have been made, a concentration profile obtained from a balloon platform using Fourier transform thermal emission spectroscopy in the far infrared. Measurements were made using the 112/cm R-Q5 branch of the rotational-torsional spectrum, with some confirmation from the 94/cm R-Q4 branch. The volume mixing ratio of H2O2 is 1.6 x 10 to the -10th at 38.4 km, decreasing to 0.6 x 10 to the -10th at 23.8 km, with uncertainties of about 16 percent. These measurements are compared to a recent stratospheric model calculation.

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