Other
Scientific paper
Dec 1986
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1986gecoa..50.2707r&link_type=abstract
Geochimica et Cosmochimica Acta, Volume 50, Issue 12, p. 2707-2717.
Other
4
Scientific paper
Cupric oxide oxidation has been employed to characterize the lignin geochemistry of Narragansett Bay sediments. Lignin concentrations throughout the estuary are low when expressed on a carbon-normalized basis, but can be characterized as enriched when expressed on a mass-normalized basis. This implies substantial dilution of the sedimentary lignin by inputs of lignin-poor carbon. Lignin concentrations do not correlate with the 13C isotopic composition of the sedimentary organic matter. These results are consistent with a sediment lignin component consisting of varying amounts of vascular plant debris and lignin-depleted organic matter, the latter originating from both marine (planktonic) and terrestrial (uncharacterized) sources. Compositional plots of lignin-derived phenols show that sediments in the upper estuary are influenced to a greater extent by gymnosperm lignin sources than those in the mid-and lower estuary. Given the extent to which the upper estuary is affected by pollution sources, inputs from anthropogenic discharges are the most likely cause of these compositional differences. However, an evaluation of processed paper products as an “anthropogenic” lignin source indicates that the lignin content of these materials is insufficient to account for the levels found in the sediments. Subsurface lignin compositions at an upper estuary site reveal that lignin originating from the inferred anthropogenic sources disappears at a depth shallower than that which would be expected based on the distribution of other trace organic pollutants (hydrocarbons and several synthetic organic compounds). We speculate that differences in either the depositional history or the degree of preservation of these two compound classes are responsible for the observed trends.
Boehm Paul D.
Brown John S.
Requejo Adolfo G.
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