Isotopic exchange between carbon dioxide and ozone via O(1D) in the stratosphere

Details Isotopic exchange between carbon dioxide and ozone via O(1D) in the stratosphere Isotopic exchange between carbon dioxide and ozone via O(1D) in the stratosphere

Jan 1991

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1991georl..18...13y&link_type=abstract

Geophysical Research Letters (ISSN 0094-8276), vol. 18, Jan. 1991, p. 13-16. Research supported by EPA.

Other

47

Atmospheric Chemistry, Carbon Dioxide, Ozone, Photochemical Reactions, Stratosphere, Oxygen Atoms, Oxygen Isotopes, Reaction Kinetics

Scientific paper

A novel mechanism for isotropic exchange between CO2 and O3 via O(1D) + CO2 - CO3(asterisk) followed by CO3(asterisk) - CO2 + O(3P). A one-dimensional model calculation shows that this mechanism can account for the enrichment in O-18 in the stratospheric CO2 observed by Gamo et al. (1989), using the heavy O3 profile observed by Mauersberger (1981). The implications of this mechanism for other stratospheric species and as a source of isotopically heavy CO2 in the troposphere are briefly discussed.

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