Infrared Spectroscopy of Metal Ligand and Metal Oxide Ligand Complexes

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Mini-Symposium: Metal Containing Molecules

Scientific paper

Metal ligand and metal oxide ligand complexes are generated in a laser vaporization/supersonic expansion cluster source and are mass selected and studied using infrared spectroscopy in the 600-4000 wn region using a tunable infrared OPO. Several different systems are investigated and some show evidence for intracluster reactions to form metal oxide species or coupling of coordinating ligands. In particular the V(CO2)n+ system shows evidence for the onset of in intracluster reaction at n=7 as evidenced by the sudden appearance of a band at 1800 wn. DFT calculations are performed in support of this work and several possible interpretations of the experimental data will be presented.

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