Hafnium isotope evidence for `conservative' element mobility during subduction zone processes

Details Hafnium isotope evidence for `conservative' element mobility during subduction zone processes Hafnium isotope evidence for `conservative' element mobility during subduction zone processes

Oct 2001

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2001e%26psl.192..331w&link_type=abstract

Earth and Planetary Science Letters, Volume 192, Issue 3, p. 331-346.

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Scientific paper

The high field strength elements (HFSE) play a critical role in the interpretation of chemical variation within subduction-related magmas by providing an assumed mantle-dominated `baseline' from which enrichments in many other slab-derived elements may be gauged. Of the HFSE, hafnium is unique in combining the characteristics of HFSE chemistry with a powerful isotopic tracer and should, in theory, allow the delineation of mantle domains and help constrain the timing of melt depletion processes. A detailed Hf isotope study of oceanic arc lavas and paired arc/back-arc settings has been conducted. Here we show, contrary to expectations, that the Hf isotopic compositions of arc lavas are always displaced significantly from their co-existing back-arc spreading centres which can be considered to sample the local mantle. This is true not only of those arcs in which direct sediment melting or AFC-like processes within the crust are implicated, but also in low-K tholeiitic arcs where hydrous fluids are believed to be the dominant medium of slab-to-mantle transport. This observation calls into question the concept of `conservative' or `immobile' elements and suggests that some transfer of material from the subducting slab into the sub-arc mantle wedge probably occurs for almost all elements. These conclusions have significant implications for models of arc geochemistry.

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