Formation of Excited H_3O States by Charge Transfer from Cs

Details Formation of Excited H_3O States by Charge Transfer from Cs Formation of Excited H_3O States by Charge Transfer from Cs

Jun 2009

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2009mss..confefa03d&link_type=abstract

"International Symposium On Molecular Spectroscopy, 64th Meeting, Held 22-26 June, 2009 at Ohio State University. http://molspec

Mathematics

Probability

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Scientific paper

Charge transfer (CT) probability between Cs and H_3O^{+} was studied. In the experiment a Rydberg type H_3O molecule is formed in electronically excited state after CT from Cs, following by the dissociation to H_2O+H. However it is not clear which excited state is a precursor of the dissociation. Electronic structure of H_3O molecule was investigated by ab initio methods. Couplings between initial and target states were calculated, and charge transfer probabilities were estimated. Calculations show that 4s Rydberg state of H_3O molecule is the most likely state to be populated in the experiment.

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