Computer Science
Scientific paper
May 1998
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1998e%26psl.158...31d&link_type=abstract
Earth and Planetary Science Letters, vol. 158, Issue 1-2, pp.31-38
Computer Science
14
Rhyolites, Peralkalic Composition, Water, Melts, Viscosity, Plastic Flow, Models
Scientific paper
The viscosities of a series of water-bearing peralkaline rhyolitic melts have been experimentally determined. The dry melt compositions are composed of a series of additions of Na 2 O to a metaluminous base composition. The melts, initially hydrated at high pressures and quenched isobarically, have been prepared by cutting and polishing, then reheating across the glass transition at 1 atm where they are annealed to a relaxed metastable state and then investigated dilatometrically using micropenetration methods. The measurements have been performed in the viscosity range of 10 8.5 -10 11.5 Pa s which corresponds to temperatures in the range of 675-220°C for these compositions. Despite the relatively low viscosities of dry peralkaline melts in comparison with metaluminous melts of similar SiO 2 content, the viscosities of peralkaline rhyolitic melts also decrease strongly and non-linearly with the addition of water. The resulting viscosity-temperature relationships for water-bearing peralkaline rhyolitic melts are shifted to much lower temperatures such that glass transition temperatures for moderate cooling rates correspond to extraordinarily low temperatures. A model is presented for the calculation of melt viscosities in the range of 10 8.5 -10 11.5 Pa s for peralkaline rhyolites with up to 7 wt% H 2 O. The very fluid nature of these peralkaline rhyolites over a wide range of water contents may facilitate a very efficient degassing history of glassy peralkaline rhyolites in nature. Efficient degassing might explain the apparent contradiction of the presence of common water-rich melt inclusions in phenocryst phases hosted in water-free glassy rhyolites, versus the absence of vesicular layers or textural evidence for a vesicular past for the glassy rocks.
Dingwell Donald B.
Hess Kai-Uwe
Romano Christian
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