Extinction calculations of multi-sphere polycrystalline graphitic clusters - A comparison with the 2175 AA peak and between a rigorous solution and discrete-dipole approximations

Details Extinction calculations of multi-sphere polycrystalline graphitic clusters - A comparison with the 2175 AA peak and between a rigorous solution and discrete-dipole approximations Extinction calculations of multi-sphere polycrystalline graphitic clusters - A comparison with the 2175 AA peak and between a rigorous solution and discrete-dipole approximations

2001-11-14

arxiv.org/abs/astro-ph/0111274v2

Astron.Astrophys. 411 (2002) 481

Astronomy and Astrophysics

Astrophysics

Corrections added in accordance with suggestions by the referee. 12 pages, 12 figures. Accepted for publication in Astronomy &

Scientific paper

10.1051/0004-6361:20020125

Certain dust particles in space are expected to appear as clusters of individual grains. The morphology of these clusters could be fractal or compact. In this paper we study the light scattering by compact and fractal polycrystalline graphitic clusters consisting of touching identical spheres. We compare three general methods for computing the extinction of the clusters in the wavelength range 0.1 - 100 micron, namely, a rigorous solution (Gerardy & Ausloos 1982) and two different discrete-dipole approximation methods -- MarCODES (Markel 1998) and DDSCAT (Draine & Flatau 1994). We consider clusters of N = 4, 7, 8, 27,32, 49, 108 and 343 particles of radii either 10 nm or 50 nm, arranged in three different geometries: open fractal (dimension D = 1.77), simple cubic and face-centred cubic. The rigorous solution shows that the extinction of the fractal clusters, with N < 50 and particle radii 10 nm, displays a peak within 2% of the location of the observed interstellar extinction peak at ~4.6 inverse micron; the smaller the cluster, the closer its peak gets to this value. By contrast, the peak in the extinction of the more compact clusters lie more than 4% from 4.6 inverse micron. At short wavelengths (0.1 - 0.5 micron), all the methods show that fractal clusters have markedly different extinction from those of non-fractal clusters. At wavelengths > 5 micron, the rigorous solution indicates that the extinction from fractal and compact clusters are of the same order of magnitude. It was only possible to compute fully converged results of the rigorous solution for the smaller clusters, due to computational limitations, however, we find that both discrete-dipole approximation methods overestimate the computed extinction of the smaller fractal clusters.

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