Effects of anisotropic interaction on collision-induced absorption by pairs of linear molecules

Details Effects of anisotropic interaction on collision-induced absorption by pairs of linear molecules Effects of anisotropic interaction on collision-induced absorption by pairs of linear molecules

Jun 1992

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1992phrvl..68.3686b&link_type=abstract

Physical Review Letters (ISSN 0031-9007), vol. 68, no. 25, June 22, 1992, p. 3686-3689.

Statistics

Computation

12

Absorption Spectra, Anisotropy, Carbon Monoxide, Molecular Absorption, Molecular Collisions, Nitrogen, Intermolecular Forces, Perturbation Theory

Scientific paper

Calculations of collision-induced absorption spectral moments gamma1 and alpha1 for N2 and CO2 molecular pairs are presented which, for the first time, fully account for the anisotropic components of the inter-molecular potentials. The results of these rigorous computations, performed at selected temperatures, are compared with approximations based on the perturbative approach and the infinite-order sudden approximation. In this way both important aspects of the effects of an anisotropic interaction and the ability of these two approximations to take them into account are demonstrated.

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