Covariance mapping - A correlation method applied to multiphoton multiple ionization

Details Covariance mapping - A correlation method applied to multiphoton multiple ionization Covariance mapping - A correlation method applied to multiphoton multiple ionization

Nov 1989

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1989sci...246.1029f&link_type=abstract

Science (ISSN 0036-8075), vol. 246, Nov. 24, 1989, p. 1029-1031. Research supported by SERC.

Mathematics

107

Carbon Monoxide, Covariance, Mapping, Photoionization, Time Of Flight Spectrometers, Ultrashort Pulsed Lasers, Autocorrelation, Matrices (Mathematics), Molecular Ions, Picosecond Pulses

Scientific paper

Covariance mapping allows hidden correlation in a highly fluctuating signal which are lost in a conventional averaging procedure to be revealed unambiguously. Here, an experiment is described in which the covariance approach is used to analyze the fragmentation pattern of molecules after multiple ionization by an intense subpicosecond laser. In this experiment, the covariance is displayed in the form of a two- or three-dimensional map of competing fragmentation channels with axes given by ion time of flight.

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