Other
Scientific paper
Jun 1987
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1987gecoa..51.1651s&link_type=abstract
Geochimica et Cosmochimica Acta (ISSN 0016-7037), vol. 51, June 1987, p. 1651-1664.
Other
10
Carbon Dioxide, Clathrates, Methane, Raman Lasers, Raman Spectra, Water, Geophysical Fluids, Phase Diagrams, Room Temperature
Scientific paper
A set of 33 synthetically produced CO2-CH4-H2O fluid inclusions in quartz have been subjected to microthermometry (MT) and laser Raman microprobe (LRM) spectroscopy. The inclusions encompass an aqueous liquid, a CO2-CH4 supercritical carbonic fluid, and graphite. A method is presented by means of which MT data for these inclusions can be projected within the CO2-CH4 binary phase diagram to infer CO2:CH4 ratios in the carbonic fluid, taking into account the formation of CO2-CH4 clathrate during MT analysis. Comparison of LRM analyses on the bulk carbonic fluid and the residual carbonic fluid confirm the preferential partitioning of CH4 in the clathrate.
Dill Pasteris Jill
Seitz Jeffery C.
Wopenka Brigitte
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