Bonding in silicates: an assessment of bonding in orthopyroxene

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The molecular orbital and crystal field theories are compared and their applicabilities to bonding in silicates are discussed, A molecular orbital bonding model is favoured for orthopyroxene since bonding in both tetrahedral and non-tetrahedral sites within the crystal structure can be described and accommodated by the theory. It is suggested that Fe located in M 2 sites has more electron delocalisation (or covalence) associated with it than Fe located in the M 1 site. Order-disorder phenomena in orthopyroxene are discussed in relationship to Mueller's (1970) two-step exchange mechanism, whereby the first step corresponds to vacancy activation and the second step to exchange of Fe between an `octahedral' site and a vacancy.

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