Bimolecular Reactions of a Different Color: CH3D + Chlorine with Varied Photolysis Wavelengths

Details Bimolecular Reactions of a Different Color: CH3D + Chlorine with Varied Photolysis Wavelengths Bimolecular Reactions of a Different Color: CH3D + Chlorine with Varied Photolysis Wavelengths

Jun 2011

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2011mss..confetb09b&link_type=abstract

"International Symposium On Molecular Spectroscopy, 66th Meeting, Held 20-24 June, 2011 at Ohio State University. http://molspec

Computer Science

Dynamics

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We examine the effect varying the collision energy has on the bimolecular reaction of CH3D and chlorine. A Raman shifting cell pumped at 355 nm and filled with either hygrogen or methane gas provides, in discrete steps, light to photolyze Cl_2. This imparts bewteen 600 and 2000 Cm-1 of collision energy to our system. By also adding C-H vibrational overtone excitation, around 6000 Cm-1, we can compare to previous, fixed-photolysis energy studies from our reseach group. We seek to elucidate the role translational energy (collision energy) plays in this reactive system.

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