Computer Science – Sound
Scientific paper
Sep 1993
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1993georl..20.1795a&link_type=abstract
Geophysical Research Letters (ISSN 0094-8276), vol. 20, no. 17, p. 1795-1798.
Computer Science
Sound
22
Atmospheric Chemistry, Balloon-Borne Instruments, Chlorine Oxides, In Situ Measurement, Midlatitude Atmosphere, Ozonometry, Atmospheric Sounding, Nitrogen Oxides
Scientific paper
In situ measurements of chlorine oxide (ClO) obtained on 31 March 1991 with a new balloon-borne instrument are compared to results from a photochemical model which incorporates hydrolysis of N2O5 on sulfate aerosols. With the addition of this process, there is better agreement between calculation and measurement over most of the profile, except below 20 km where observed ClO is greater by as much as a factor of four. In a model which is constrained to reproduce the observed ClO below 20 km, ozone loss by catalytic cycles involving halogen oxides becomes larger than that from NO(x), which would dominate under gas-phase or standard heterogeneous conditions.
Anderson James G.
Avallone Linnea M.
Brune William H.
Dessler Andrew E.
Salawitch Ross J.
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