A theoretical treatment of the absorption spectra of all-benzenoid hydrocarbons

Astronomy and Astrophysics – Astronomy

Scientific paper

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Astrochemistry, Molecular Data, Ism: Lines And Bands, Ism: Molecules, Infrared: Ism

Scientific paper

The class of compounds known as the all-benzenoid polycyclic aromatic hydrocarbons (ABPAHs) are treated with time-dependent density functional theory (TDDFT) and a modified Hückel theory to determine how large an ABPAH must be before it is found to absorb strongly in the visible region that corresponds to the bluest of the diffuse interstellar bands (DIBs). The first six ABPAHs are treated with TDDFT using the B3LYP functional to determine their excitation energies. A two-parameter Hückel theory is adopted to deal with those systems too large to be addressed with TDDFT. The transitions are calculated and fitted to experimental data. An ABPAH system with 84 carbons and 14 all-benzenoid rings is found to be the first carrier to absorb strongly in the region where DIBs are observed.

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