Solid oxide electrolyte emf cell determination of the standard free energy of Cr 2 O 3 and applications to chromium-bearing mineral systems

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Emf measurements are reported on cells using a thoria-yttria solid oxide electrolyte. The measured potentials from two cells, Cr, Cr 2 O 3 ¦ThO 2 -Y 2 O 3 ¦Co, CoQ and Cr, Cr 2 O 3 ¦ThO 2 -Y 2 O 3 ¦ Mn, MnO, were used to calculate the standard Gibbs free energy of formation of Cr 2 O 3 in the temperature range 875-1275°C. The two separate series of measurements are in good agreement with critically assessed data from the literature based on gas equilibration and calorimetric results. A summary of solid oxide electrolyte studies on mineral systems is presented with special attention paid to chromium-bearing solutions or compounds. The application of this experimental technique in investigating thermodynamic properties of chromium minerals is discussed.

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