The rotational excitation of carbon monoxide by hydrogen atom impact

Details The rotational excitation of carbon monoxide by hydrogen atom impact The rotational excitation of carbon monoxide by hydrogen atom impact

Feb 1975

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1975rspsa.342..191c&link_type=abstract

Royal Society (London), Proceedings, Series A, vol. 342, no. 1629, Feb. 25, 1975, p. 191-207. NSF-supported research.

Mathematics

86

Atomic Collisions, Carbon Monoxide, Hydrogen Atoms, Molecular Excitation, Molecular Rotation, Scattering Cross Sections, Adiabatic Equations, Coupling, Electron Scattering, Intermolecular Forces, Mathematical Models, Molecular Collisions, Particle Interactions, Potential Theory

Scientific paper

The present work represents a quantal study of the rotational excitation of carbon monoxide in collision with atomic and molecular hydrogen. A rigorous close-coupling formulation for a rigid rotator model is used to assess the reliability of the adiabatic approximation for electron-molecule collisions. The usefulness of two close-coupling approximations, that of Rabitz (1972) and that of McGuire & Kouri (1974), is investigated. These approximations achieve a substantial reduction in the number of coupled channels and may be especially valuable for the description of collisions between pairs of molecules.

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